

We study the dynamical behavior of a Lennard-Jones fluid
using constant-energy molecular dynamics simulations. The
system is studied at several points of the
density-temperature phase diagram. Power spectra of
instantaneous temperature and pressure show a two-regime
power-law 1/f^a behavior. Rescaled range analysis (Hurst
test) reveals also this two-regime behavior with strong
memory effects for short times and gradual loss of memory at
longer times. The dependence of memory on system density and
temperature is discussed. By analyzing the Mean Square
Displacement (MSD) of the atoms, the two-regime behavior is
found to be associated with two kinds of atomic motion:
vibrational (high frequency) and diffusional (low
frequency). Characteristic times extracted from MSD
calculations are in agreement with times deduced from
spectral analysis. The system exhibits high-dimensional
chaotic dynamics which is difficult to distinguish from
stochastic behavior. We calculate the largest Lyapunov
exponent of the system and discuss algorithms for the
computation of the full Lyapunov spectrum.
[MM.002] Non-reversiblity in periodically driven flows by viscous dephasing
Bruno Eckhardt (Fachbereich Physik, Philipps Universitaet Marburg, Germany), Erwan Hascoet (Department of Aeronautics, Imperial College, London)
We show that in generic situations a reversible periodic
driving of a low-Reynolds number flow will not result in a
reversible flow field. In the famous experiment of GI Taylor
with a blob of dye between concentric cylinders only a
single eigenmode of the Stokes operator is involved and
reversibility is assured. In generic situations several
modes are present and since each eigenmode responds with a
phase delay that depends on its eigenvalue and the driving
frequency, not all modes will be in phase anymore. Such a
viscous dephasing then breaks time reversal symmetry. The
general theory is illustrated for 2-d vortex patterns that
can be generated in current driven flows in a magnetic
field.
[MM.003] Lagrangian chaos and resonance phenomena in Stokes flows
Dmitri Vainchtein (University of California Santa Barbara), Neishtadt Neishtadt (Space Research Institute, Moscow, Russia), Igor Mezic (University of California Santa Barbara)
We discuss the Lagrangian chaos in a Stokes flow between two
counter-rotating coaxial cylinders with the angular
velocities depending on the coordinate along the axis. The
streamlines of the unperturbed system are closed and the
flow is regular. However, if an additional weak flow
parallel to the axis is applied, Lagrangian chaos develops.
We show that this phenomenon is caused by quasi-random
changes (jumps) in the adiabatic invariant of the flow,
which occur when streamlines cross the resonance surface. We
demonstrate that the accumulation of the jumps leads to the
diffusion of adiabatic invariant. For multiple resonance
crossings. We discuss the statistical properties of the
jumps. We study the long-time mixing properties of the flow
and compare our results with numerical simulations.
[MM.004] Mode-locking of chemical pulses in an advection-reaction-diffusion system
Matt Paoletti, Tom Solomon (Department of Physics, Bucknell University, Lewisburg, PA 17837 USA)
We present results of experimental studies of the
propagation of chemical fronts in a chain of oscillating
vortices, a system in which mixing of passive
impurities is chaotic. A variation of the photosensitive
Belousov-Zhabotinsky chemical reaction is used in which a
reaction pulse can be triggered with a silver wire. The
speed at which this pulse propagates through the vortex
chain is measured and compared with recent
theories(M. Cencini, A. Torcini, D. Vergni and A.
Vulpiani, Phys. Fluids 15, 679 (2003)) for front propagation
in a similar flow. Several mode-locked regimes are observed
in which the pulse propagates an integer number of vortex
widths in an integer number of oscillation periods.
Measurements of the widths of these locking regimes are made
as a function of the oscillation amplitude, revealing
classic Arnol’d tongue behavior.
[MM.005] Chemical pulses and superdiffusive transport in an oscillating-drifting vortex chain
Tom Solomon, Matt Paoletti (Department of Physics, Bucknell University, Lewisburg, PA 17837 USA)
We discuss experimental and numerical studies of transport
and pulse propagation in an alternating vortex chain that
can both oscillate and drift. Previous studies have shown
that transport in the oscillating vortex is chaotic, with a
variance that grows linearly with time; i.e., the transport
is diffusive in nature. The addition of drifting to the
vortex chain allows for superdiffusive transport with a
variance that grows faster than linearly with time. We
present particle-tracking data for transport in this system,
along with experimental studies of the propagation of
chemical pulses for the oscillating/drifting vortex chain.
[MM.006] Self-consistent chaotic mixing of active impurities in a vortex chain
Louis McLane, Julie Jakoboski, Tom Solomon (Department of Physics, Bucknell University, Lewisburg, PA 17837 USA)
Experiments are performed on the effects of active mixing on
the dynamics of a vortex chain. The process is called
“self-consistent” because of its circular nature: the mixing
affects the time-dependence of the flow which, in turn,
affects the mixing. The flow is forced
magnetohydrodynamically -- an electrical current passes
through a salt-water solution and interacts with an
alternating magnetic field to generate a chain of vortices.
The system is forced with a current below that for
time-dependent oscillations. A more concentrated salt
solution is injected as the active impurity. An instability
arises in which blobs of more- and less-concentrated salt
solution are advected around the vortices, causing
oscillations in the vortex boundaries and leading to chaotic
mixing of impurities between vortices.
[MM.007] Simulations of the Reaction-Diffusion System demonstrating the Transition from Purely Temporal to Spatio-Temporal Chaos
Thomas Olsen, Yu Hou, Collin Trail (Lewis amp; Clark College, Portland, OR), Richard Wiener (Pacific University, Forest Grove, OR)
The Reaction-Diffusion model (H. Riecke and H.-G.
Paap, Europhys. Lett. \textbf14), 1235 (1991).has been
applied to a wide variety of pattern forming systems. It
correctly predicted a period doubling cascade to chaos in
Taylor-Couette flow with hourglass geometry(Richard
J. Wiener \textitet al), Phys. Rev. E \textbf55, 5489
(1997).. We have conducted a series of such simulations,
varying the length of the system. This has enabled us to
study the transition from a purely temporal chaos of the
formation of new pairs of Taylor Vortices at a single
location, to a spatio-temporal chaos of formation across a
range of locations. Application to anticipated experiments
will be discussed.
[MM.008] Ruelle-Takens scenario in a confined two-dimensional flow
Gertjan Van Heijst, D. Molenaar, H.J.H. Clercx (Physics Department, Eindhoven University of Technology, Eindhoven, The Netherlands)
Ruelle, Takens and Newhouse (Commun. Math. Phys. 20,
1971; 64, 1978) argued that, as a function of an
external parameter, the route to chaos in a fluid flow is a
transition sequence leading from stationary (S) to single
periodic (P), double periodic (QP_2), triple periodic
(QP_3) and, possibly, quadruply periodic (QP_4) motions,
before the flow becomes chaotic (C). However, the
quasi-periodic motions with 3 or 4 incommensurate
frequencies were shown to be unstable with respect to small
perturbations and may, hence, not be observed at all.
Using direct numerical simulations, we show that the route
to chaos in a forced two-dimensional flow, confined to a
square domain with two no-slip boundaries, essentially
follows a Ruelle-Takens scenario. In this flow the kinematic
viscosity \nu serves as the control parameter. Its value
is decreased in discrete steps, whilst keeping the amplitude
of a time-independent external forcing fixed. As such, the
sequence encountered in our simulations, within the interval
1/700\geq\nu\geq 1/1700, is S\rightarrow P\rightarrow
QP_2\rightarrow QP_3\rightarrow C, where each transition
corresponds to a Hopf bifurcation. These motions are
analyzed in terms of their fundamental frequencies and a
phase-space reconstruction.
[MM.009] Reynolds number dependence of fluid mixing in the partitioned-pipe mixer
Yoshinori Mizuno, Mitsuaki Funakoshi (Graduate School of Informatics, Kyoto University)
Reynolds number dependence of chaotic mixing of fluids in
the partitioned-pipe mixer (PPM) is studied by using
numerically obtained velocity fields. We found that
transport barriers once expand as the Reynolds number,
R_e, is increased. Although they tend to disappear with
increase in R_e, some of them remain for relatively large
R_e in some cases in which a geometrical condition of the
system is changed. Existence of the barriers can be related
to dimensionality of the velocity field. On mixing in the
chaotic region, we found that a high shear region apart from
the rigid wall appears as R_e is increased enough. This
appearance of a high shear region is expected to enhance
mixing efficiency in the chaotic region.
[MM.010] Dynamic Subgrid-Scale Drag Modeling for Turbulent Flow Over Fractal Trees
Stuart Chester, Charles Meneveau, Marc Parlange (Johns Hopkins University)
LES ideas, in particular the dynamic model (Germano et al. 1991), are extended and applied to the problem of SGS drag modeling for flow over trees. The SGS branch drag coefficient is determined as in dynamic LES by enforcing model consistency amongst SGS branches and the smallest resolved branches, and assuming scale invariance of the drag coefficient. The formulation allows for dependence of the drag coefficient on the geometrical configuration of a given branch (e.g. orientation relative to the incoming flow), which results in a linear system for the drag coefficients. Results are obtained by performing LES of high-Re turbulent flow over idealized leafless, self-similar fractal trees as a test case. A posteriori tests show that the dynamic drag coefficients are stable in many cases, although less robust coefficients are associated with trees with a high degree of branching. The total SGS drag force is observed to be a significant fraction of the total drag force on the tree, highlighting the importance of the drag model. Observed nontrivial dependence of the dynamically obtained drag coefficients on branch orientation will also be presented.