Pressure-Induced Oxygen Ordering Effects in High-T _c Superconductors*

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Session Q09 - HTSC: STRUCTURES AND DEFECTS
Mixed session, Friday morning, March 24, 8:00
Ballroom A5, San Jose Convention Center

[Q09.13] Pressure-Induced Oxygen Ordering Effects in High-T _c Superconductors*

A.-K. Klehe,C. Looney,J.S. Schilling (Dept. Physics, Washington Univ., St. Louis, MO),H. Takahashi,N. Mori (Inst. Sol. State Physics, Univ. of Tokyo (Japan)),Y. Shimakawa,Y. Kubo,T. Manako (NEC Corp., Tsukuba (Japan))

The dependence of the superconducting transition temperature on pressure T _c (P) has been determined for Tl _2 Ba _2 CuO _6+\delta and TlSr _2 CaCu _2 O _7-\delta at different oxygen concentrations. The pressure derivative dT _c /dP is found to depend strongly on the temperature at which the hydrostatic He-gas pressure is applied. This result is believed to originate from pressure-induced ordering of oxygen defects at ambient temperature, a process which is prevented by sluggish kinetics if the pressure is changed at low temperatures (50 K). A detailed study of both T _c and the Hall number n _H as function of pressure, temperature and time reveals distinct ''fast'' and ''slow'' relaxation processes in the oxygen defect subsystem. Related oxygen ordering effects may be quite common in the high-T _c oxides. Evidence is discussed for the existence of ''fast'' oxygen ordering processes in YBa _2 Cu _3 O _7-y which may be responsible for ''transient photo-induced superconductivity''.

*Research supported by NSF grant DMR-9208531.

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